Specific Heat Anomalies in Solids Described by a Multilevel Model



Document title: Specific Heat Anomalies in Solids Described by a Multilevel Model
Journal: Brazilian journal of physics
Database: PERIÓDICA
System number: 000392506
ISSN: 0103-9733
Authors: 1
1
1
1
Institutions: 1Universidade Estadual Paulista "Julio de Mesquita Filho", Instituto de Geociencias e Ciencias Exatas, Rio Claro, Sao Paulo. Brasil
Year:
Season: Abr
Volumen: 46
Number: 2
Pages: 206-212
Country: Brasil
Language: Inglés
Document type: Artículo
Approach: Experimental, analítico
English abstract In the field of condensed matter physics, specific heat measurements can be considered as a pivotal experimental technique for characterizing the fundamental excitations involved in a certain phase transition. Indeed, phase transitions involving spin (de Souza et al. Phys. B Condens. Matter 404, 494 (2009) and Manna et al. Phys. Rev. Lett. 104, 016403 (2010)), charge (Pregelj et al. Phys. Rev. B 82, 144438 (2010)), lattice (Jesche et al. Phys. Rev. B 81, 134525 (2010)) (phonons) and orbital degrees of freedom, the interplay between ferromagnetism and superconductivity (Jesche et al. Phys. Rev. B 86, 020501 (2012)), Schottkylike anomalies in doped compounds (Lagos et al. Phys. C Supercond. 309, 170 (1998)), electronic levels in finite correlated systems (Macedo and Lagos J. Magn. Magn. Mater. 226, 105 (2001)), among other features, can be captured by means of high-resolution calorimetry. Furthermore, the entropy change associated with a first-order phase transition, no matter its nature, can be directly obtained upon integrating the specific heat over T , i.e.,C(T )/T , in the temperature range of interest. Here, we report on a detailed analysis of the two-peak specific heat anomalies observed in several materials. Employing a simple multilevel model, Mariano de Souza mariano@rc.unesp.br 1 Departamento de F´ısica, IGCE, Unesp - Univ Estadual Paulista, 13506-900, Rio Claro, SP, Brazil 2 Departamento de F´ısica e Qu´ımica, Unesp - Univ Estadual Paulista, 15385-000, Ilha Solteira, SP, Brazil 3 Present address: Institute of Semiconductor and Solid State Physics, Johannes Kepler University Linz, Linz, Austria varying the spacing between the energy levels i = (Ei − E0) and the degeneracy of each energy level gi, we derive the required conditions for the appearance of such anomalies. Our findings indicate that a ratio of 2/1 ≈ 10 between the energy levels and a high degeneracy of one of the energy levels define th
Disciplines: Física y astronomía
Keyword: Física de materia condensada,
Calor específico,
Función de partición,
Efectos de correlación
Keyword: Physics and astronomy,
Condensed matter physics,
Specific heat,
Partition function,
Correlation effects
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