Increase of Curie temperature with La doping in the double perovskite Sr2−yLayFeMoO6 within an electronic correlation approach



Título del documento: Increase of Curie temperature with La doping in the double perovskite Sr2−yLayFeMoO6 within an electronic correlation approach
Revue: Revista mexicana de física
Base de datos: PERIÓDICA
Número de sistema: 000426076
ISSN: 0035-001X
Autores: 1
1
1
1
5
Instituciones: 1Universidad Nacional Autónoma de México, Instituto de Investigaciones en Materiales, Morelia, Michoacán. México
2Universidad Michoacana de San Nicolás de Hidalgo, Facultad de Ciencias Físico-Matemáticas, Morelia, Michoacán. México
3Universidad Michoacana de San Nicolás de Hidalgo, Facultad de Biología, Morelia, Michoacán. México
4Universidad Nacional Autónoma de México, Instituto de Geofísica, Morelia, Michoacán. México
5Universite Grenoble Alpes, Grenoble, Isere. Francia
Año:
Periodo: Mar-Abr
Volumen: 64
Número: 2
País: México
Idioma: Inglés
Tipo de documento: Artículo
Enfoque: Analítico, teórico
Resumen en inglés The double perovskite compound Sr2FeMoO6 has a half-metallic ferromagnetic character and a high Curie temperature (420 K). Fe-Mo usually present some degree of disorder in either Fe or Mo ions, it is therefore fundamental to understand the role of electronic and structural parameters controlling the half-metallic character together with a Curie temperature as high as possible. We replaced divalent Sr2+ by trivalent La3+ ions in Sr2FeMoO6 system to observe the Curie temperature behavior. We present an electronic approach using the Green’s functions and the renormalization perturbation expansion method, with localized Fe-spins and conduction Mo-electrons interacting with the local spins via a double-exchange-type mechanism. We also include the electronic correlations among the conduction electrons within a mean-field approximation. Our results show the density of states and the Curie temperature behavior when La concentration increases for the Sr 2−y La y FeMoO6 system
Disciplinas: Física y astronomía
Palabras clave: Física,
Perovskitas dobles,
Semimetalicidad,
Temperatura de Curie
Keyword: Physics,
Double perovskites,
Half-metallicity,
Curie temperature
Texte intégral: Texto completo (Ver HTML) Texto completo (Ver PDF)